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Rhodium-catalyzed enantioselective conjugate addition of arylboronic acids to dihydronitronaphthalenes

Published in: Journal, Volume : 354, Issue : 13, Pages : 2433-2437, S2433/1-S2433/39

DOI : 10.1002/adsc.201200241

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A highly enantioselective (up to 91% ee) rhodium-catalyzed asym. addition of arylboronic acids has been achieved leading to the challenging dihydro-3-nitronaphthalenes using one equivalent of phosphoramidite ligand to rhodium catalyst. A concise formal asym. synthesis of the dopamine D1 agonist, dihydrexidine was accomplished using the method.

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